https://doi.org/10.1051/epjconf/20134102021
Fragmentation Control of a Polyatomic Molecule by fully determined Laser-Fields
1 Photonics Institute, Vienna University of Technology, A-1040 Vienna, Austria
2 Institute of Optics and Quantum Electronics, D-07743 Jena, Germany
3 Institute of Theoretical Physics, Vienna University of Technology, A-1040 Vienna, Austria
4 Department of Physics and Astronomy, Vanderbilt University, Nashville, Tennessee 37235, USA
5 Department of Chemistry, School of Science, The University of Tokyo, Tokyo 113-0033, Japan
6 State Key Laboratory on Integrated Optoelectronics, Changchun 130012, China
a e-mail: markus.kitzler@tuwien.ac.at
Strong-field control of acetylene fragmentation by fully determined few-cycle laser pulses is demonstrated. The control mechanism is shown to be based on electron recollision and inelastic ionization from inner-valence molecular orbitals.
© Owned by the authors, published by EDP Sciences, 2013
This is an Open Access article distributed under the terms of the Creative Commons Attribution License 2.0, which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.