https://doi.org/10.1051/epjconf/20134105001
Exploring Higher-Lying Electronic States of a Molecular Switch by Coherent Triggered-Exchange 2D Electronic Spectroscopy
Institut für Physikalische und Theoretische Chemie, Universität Würzburg, Am Hubland, 97074 Würzburg, Germany
a e-Mail: brixner@phys-chemie.uni-wuerzburg.de
We use pump-repump-probe transient absorption spectroscopy to investigate the role of higher-lying electronic states in the photochemistry of a molecular switch. Moreover, replacing the pump pulse by a pulse-shaper-generated phase-stable double pulse, triggered-exchange two-dimensional (TE2D) electronic spectroscopy is established in the visible regime.
© Owned by the authors, published by EDP Sciences, 2013
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