Photonic Time-Stretch Spectroscopy for Multiplex Stimulated Raman Scattering
1 CNR-IFN and Dipartimento di Fisica, Politecnico di Milano, P.za L. da Vinci 32, 20133 Milano, Italy
2 Center for Nano Science and Technology@PoliMi, Istituto Italiano di Tecnologia, Via Giovanni Pascoli 70/3, 20133 Milano, Italy
* Corresponding author: firstname.lastname@example.org
Published online: 16 April 2019
Stimulated Raman scattering spectroscopy enables label-free molecular identification, but its broadband implementation is technically challenging. We experimentally demonstrate a novel approach to multiplex stimulated Raman scattering based on photonic time stretch. A telecom fiber stretches the broadband femtosecond Stokes pulse after the sample to ∼15ns, mapping its spectrum in time. The signal is sampled through a fast oscilloscope, providing single-shot spectra at 80-kHz rate. We demonstrate high sensitivity in detecting the Raman vibrational modes of various samples over the entire high-frequency C-H stretching region. Our results pave the way to high-speed broadband vibrational imaging for materials science and biophotonics.
© The Authors, published by EDP Sciences, 2019
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