Simulating exciton migration and annihilation dynamics in higher order spectroscopies of a molecular trimer
1 Photonics Institute, TU Wien, GuBhausstraße 27-29, 1040 Vienna, Austria
2 Institute of Physics, Faculty of Mathematics and Physics, Charles University, Ke Karlovu 5, Prague 121 16, Czech Republic
3 Professur für Dynamische Spektroskopien, Fakultät für Chemie, Technische Universität München, Lichtenbergstr. 4, D-85748, Garching b. München, Germany
* Corresponding author: email@example.com
Published online: 16 April 2019
We present simulations of 3rd and 5th order multidimensional time-dependent signals of a molecular trimer. The developed model allows for the simulation of both signal types within one theoretical framework. We therefore extended standard Redfield theory of exciton migration by a new term to include the process of exciton-exciton annihilation.
© The Authors, published by EDP Sciences, 2019
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